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장소 E6-2, #1323 
일시 2016/1/26, 2PM 
연사 Dr. Sergei V. Kalinin (Center for Nanophase Materials Sciences, Oak Ridge National Laboratory) 

Electrochemistry on Nano- and Atomic Levels: Scanning Probe Microscopy Meets Deep Data

 

Jan. 26 (Tue), 2PM,  E6-2. #1323
Dr. Sergei V. Kalinin,  Center for Nanophase Materials Sciences, Oak Ridge National Laboratory

 

Structural and electronic properties of oxide surfaces control their physical functionalities and electrocatalytic activity, and are currently of interest for energy generation and storage applications. In this presentation, I will discuss several examples of high-resolution studies of the electronic and electrochemical properties of oxide surfaces enabled by multidimensional scanning probe microscopies. On the mesoscopic scale, combination of strain- and current sensitive scanning probe microscopies allows to build nanometer-scale maps of local reversible and irreversible electrochemical activities. The use of multivariate statistical methods allows separating the complex multidimensional data sets into statistically significant components which in certain cases can be mapped onto individual physical mechanisms. I will further discuss the use of in-situ Pulsed Laser Deposition growth combined with atomic resolution Scanning Tunneling Microscopy and Spectroscopy to explore surface structures and electrochemical reactivity of oxides on the atomic scale. For SrRuO3, we directly observe multiple surface reconstructions and link these to the metal-insulator transitions as ascertained by UPS methods. On LaxCa1-xMnO3, we demonstrate strong termination dependence of electronic properties and presence of disordered oxygen ad-atoms. The growth dynamics and surface terminations of these films are discussed, along with single-atom electrochemistry experiments performed by STM. Finally, I explore the opportunities for atomically-resolved imaging and property data mining of functional oxides extending beyond classical order parameter descriptions, and giving rise to the deep data analysis in materials research. 
This research is supported by the by the U.S. Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division, and was conducted at the Center for Nanophase Materials Sciences, which is sponsored at Oak Ridge National Laboratory by the Scientific User Facilities Division, BES DOE.

 

Contact: Chan-Ho Yang, Physics Dept., (chyang@kaist.ac.kr)

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217 Mar. 16 (Fri.), 02:30 PM  E6-2. 1st fl. #1323  Dr. JinHee Kim  산화물 다층박막에서의 다양한 물리현상 file
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206 2015/09/07, 3PM  E6-2. 1st fl. #1318  Dr. Jasbinder Sanghera (U.S. Naval Research Laboratory (NRL))  Advanced Optical Materials and Devices at NRL
205 4pm, Sep. 21 (Wed.  E6-2. #2502(2nd fl.)  Dr. Henrik Johannesson , University of Gothenburg (Sweden) and Beijing Computational Science Research Center (China)  Entanglement probe of two-impurity Kondo physics
204 Sep. 29 (Thu), 4:00 PM  E6-2. #2501(2nd fl.)  Dr. Minu Kim, Institute for Basic Science, Seoul National University  Exploring the phase diagram of BaBiO3: epic voyage of just another bad trip?
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202 Nov. 04 (Fri), 3:00 PM  E6-2. #1323(1st fl.)  Dr. Dohun Kim, Department of Physics and Astronomy, SNU  Quantum information experiments using few electron spins in semiconductors
201 Nov. 04 (Fri), 1:30 PM  E6-2. #1323(1st fl.)  Dr. Jonghyun Song, Department of Physics, Chungnam National University  Exotic phenomena at oxide LaAlO3/SrTiO3 hetero-interface and their applications
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