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장소 E6-2, #1323 
일시 2016/1/26, 2PM 
연사 Dr. Sergei V. Kalinin (Center for Nanophase Materials Sciences, Oak Ridge National Laboratory) 

Electrochemistry on Nano- and Atomic Levels: Scanning Probe Microscopy Meets Deep Data

 

Jan. 26 (Tue), 2PM,  E6-2. #1323
Dr. Sergei V. Kalinin,  Center for Nanophase Materials Sciences, Oak Ridge National Laboratory

 

Structural and electronic properties of oxide surfaces control their physical functionalities and electrocatalytic activity, and are currently of interest for energy generation and storage applications. In this presentation, I will discuss several examples of high-resolution studies of the electronic and electrochemical properties of oxide surfaces enabled by multidimensional scanning probe microscopies. On the mesoscopic scale, combination of strain- and current sensitive scanning probe microscopies allows to build nanometer-scale maps of local reversible and irreversible electrochemical activities. The use of multivariate statistical methods allows separating the complex multidimensional data sets into statistically significant components which in certain cases can be mapped onto individual physical mechanisms. I will further discuss the use of in-situ Pulsed Laser Deposition growth combined with atomic resolution Scanning Tunneling Microscopy and Spectroscopy to explore surface structures and electrochemical reactivity of oxides on the atomic scale. For SrRuO3, we directly observe multiple surface reconstructions and link these to the metal-insulator transitions as ascertained by UPS methods. On LaxCa1-xMnO3, we demonstrate strong termination dependence of electronic properties and presence of disordered oxygen ad-atoms. The growth dynamics and surface terminations of these films are discussed, along with single-atom electrochemistry experiments performed by STM. Finally, I explore the opportunities for atomically-resolved imaging and property data mining of functional oxides extending beyond classical order parameter descriptions, and giving rise to the deep data analysis in materials research. 
This research is supported by the by the U.S. Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division, and was conducted at the Center for Nanophase Materials Sciences, which is sponsored at Oak Ridge National Laboratory by the Scientific User Facilities Division, BES DOE.

 

Contact: Chan-Ho Yang, Physics Dept., (chyang@kaist.ac.kr)

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155 Oct. 27th(Thu) 4PM  #1323(E6-2)  Dr. 이 강 희, KAIST, Mechnical Engineering  Terahertz Metal Optics
154 June 28 (Fri.), 13:30 PM  #1323, E6-2  Dr. Yusuke Kozuka  Magnetic domains and domain wall conduction in pyrochlore iridate thin films and heterostructures file
153 Apr. 08 (Fri.), 13:30 PM  E6-2. 1st fl. #1501  Dr. Yunkyu Bang, Chonnam National Univ.  Theoretical Overview of Iron-based superconductors and its future
152 Sep. 26 (Tue.), 11AM  #1323 (E6-2. 1st fl.)  Dr. Yukiaki Ishida / ISSP, University of Tokyo  Time-resolved ARPES study of Dirac and topological materials
151 Nov. 1 (Fri.), 02:30 PM  E6-2. 1st fl. #1323  Dr. YoungWook Kim  Squeezing the best out of 2D materials file
150 Apr. 19 (Fri.), 02:30 PM  E6-2. 1st fl. #1323  Dr. YoungWoo Nam  A family of finite-temperature electronic phase transitions in graphene multilayers file
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148 Mar. 16 (Fri.), 04:0 PM  E6-2. 1st fl. #1323  Dr. YoungDuck Kim  Van der Waals Heterostructures from Quantum Transport to Ultrafast Optoelectronics file
147 May 13 (Fri.), 1:30 PM  E6. #1501(1st fl.)  Dr. Young-Woo Son, Dept. of Physics, KIAS  Aperiodic crystals in low dimensions
146 April 11 (Wed), 4:00pm  #1323 (E6-2, 1st fl.)  Dr. Young-Sik Ra  Non-Gaussian states of multimode light generated via hybrid quantum information processing file
145 May. 12 (Fri.), 01:30 PM  E6-2. 1st fl. #1323  Dr. Young Kuk Kim  Topological Dirac insulator
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